I gave up on the Fall after Wonderful and Frightening - three duff albums in a row was enough for me - so my list is skewed towards the earlier stuff. But when they were good they were really good. In no particular order:

Gut of the Quantifier (I'm telling you now and I'm telling you this...
Winter
Leave the Capitol (All the paintings you recall, all the sidestepped cars)
Fantastic Life
The N.W.R.A. (Junior Choice played one morning, the song was 'English Scene' - mine! - they'd changed it around, added a grand piano and turned it into a love song, how they did it I don't know)