No, it is much more difficult than cut with one foot and 6/8 with the other, harp. Try it! It is like tapping a very fast waltz with one foot while tapping a reel with the other. (or a waltz with one foot and a very slow reel with the other. In any case the beat is the same and the rythm just differs between feet.)I think he did the three against two because he could do it, and most people can't--that is as a show piece. In the newsreel of his wedding he does it while playing a snatch of "Goodnight Irene". He doesn't do it as a tap dance but sitting with his legs crossed. You can see him do it.
Murray