I have most of his records, and I think Live at the Old Quarter and The Late Great Townes Van Zandt are probably the best. Also very good are Townes Vandt Zandt and Our Mother the Mountain.He was a brilliant songmaker who is deeply missed.
Since we're on favorite songs as well, I particularly love "To Live is to Fly," "Marie," "Tower Song," "I'll Be Here in the Morning," and come to think of it, most of the rest of them. I was surprised, by the way, to hear "I'll be Here in the Morning" (sung by someone else) used as the music for a University of Virginia Health System commercial when I was living in Charlottesville last year.
Dan